A Novel Strongly Spin-Orbit Coupled Quantum Dimer Magnet: Yb2Si2O7

In press in Physical Review Letters (currently on arXiv)

The quantum dimer magnet (QDM) is the canonical example of “quantum magnetism”. We report our single crystal neutron diffraction, specific heat, and ultrasound velocity work on a new QDM in the strongly spin-orbit coupled, distorted honeycomb-lattice material Yb2Si2O7. These measurements reveal a gapped singlet zero field ground state with sharp, dispersive excitations. We find a field-induced magnetically ordered phase reminiscent of a BEC phase, with exceptionally low critical fields of Hc1 ~0.4 T and Hc2 ~1.4 T. These results raise the question of how anisotropy in strongly spin-orbit coupled materials modifies the field induced phases of QDMs.